锂电池百篇论文点评（2022.2.1—2022.3.31）

doi:10.19799/j.cnki.2095-4239.2022.0209

摘要/Abstract

摘要：

该文是一篇近两个月的锂电池文献评述，以“lithium”和“batter*”为关键词检索了Web of Science从2022年2月1日至2022年3月31日上线的锂电池研究论文，共有3128篇，选择其中100篇加以评论。层状正极材料的研究集中在高镍三元材料、镍酸锂、钴酸锂和富锂相材料，其相关研究关注表面包覆层、前驱体及合成条件、循环中的结构变化。负极材料的研究重点包括对硅颗粒的包覆，具有三维结构的硅/碳、硅/锡复合材料。金属锂负极的界面构筑及三维结构设计受到重点关注和研究。固态电解质的研究主要包括对硫化物固态电解质、氧化物固态电解质、聚合物与氧化物固体电解质复合材料的合成以及相关性能研究。液态电解液方面包括适应高电压正极材料及提升金属锂负极、石墨负极电池性能的添加剂与溶剂研究。针对固态电池，复合正极制备、双层电解质结构、锂界面枝晶及副反应抑制有多篇，其他电池技术主要偏重液态锂硫电池正极设计。表征分析涵盖了锂扩散、SEI形成、硫化物电解质的电化学与化学稳定性等方面。理论模拟工作涉及三元材料掺杂、电解液物化性质以及新型固态电解质搜寻，电池中电解液与正负极的界面以及固态电解质与Li的界面均受到重点关注。

关键词: 锂电池, 正极材料, 负极材料, 电解质, 电池技术

Abstract:

This bimonthly review paper highlights 100 recent published papers on lithium batteries. We searched the Web of Science and found 3128 papers online from Feb. 1, 2022 to Mar. 31, 2022. 100 of them were selected to be highlighted. High-nickel ternary layered oxides, LiNiO₂,LiCoO₂ and Li-rich oxides as cathode materials are still under extensive investigations for surface coating, preparation of precursors and structural evolution with cycling. The methods for improving the cycling performances of Si-based anode focus on surface coating and 3D structure design of the composite Si/C and Si/Sn anodes. Metallic lithium anode is extensively studied and 3D structure design and surface reconstruction are common methods. Solid state electrolyte including oxide, sulfide and composite materials have been widely studied. Meanwhile, large efforts are still devoted to liquid electrolytes for the optimizing the electrolyte for Li or graphite anode, and the high-voltage cathode materials. For solid-state batteries, there are a few papers related to the design of composite cathode, bi-layer electrolyte, and inhibition of Li dendrite and side reactions. Other relevant works are also presented to cathode design of liquid lithium sulfur battery. The characterization techniques are focused on lithium diffusion, SEI formation, electrochemical and chemical stability of the sulfide electrolytes. Theoretical simulations are directed to the doping of ternary oxide cathode materials, physical and chemical properties of liquid electrolyte and screening of solid electrolytes. The interfaces of liquid electrolyte/electrodes and solid state electrolyte/Li are also drawn large attentions.

Key words: lithium batteries, cathode material, anode material, solid state electrolyte, battery technology

中图分类号:

TM 911

乔荣涵, 岑官骏, 申晓宇, 田孟羽, 季洪祥, 田丰, 起文斌, 金周, 武怿达, 詹元杰, 闫勇, 贲留斌, 俞海龙, 刘燕燕, 黄学杰. 锂电池百篇论文点评（2022.2.1—2022.3.31）[J]. 储能科学与技术, 2022, 11(5): 1289-1304.

Ronghan QIAO, Guanjun CEN, Xiaoyu SHEN, Mengyu TIAN, Hongxiang JI, Feng TIAN, Wenbin QI, Zhou JIN, Yida WU, Yuanjie ZHAN, Yong YAN, Liubin BEN, Hailong YU, Yanyan LIU, Xuejie HUANG. Reviews of selected 100 recent papers for lithium batteries （Feb. 1， 2022 to Mar. 31， 2022）[J]. Energy Storage Science and Technology, 2022, 11(5): 1289-1304.

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