储能科学与技术 ›› 2023, Vol. 12 ›› Issue (5): 1589-1603.doi: 10.19799/j.cnki.2095-4239.2023.0089
时文超1(), 刘宇1, 张博冕1, 李琪2(), 韩春华1, 麦立强1()
收稿日期:
2023-02-22
修回日期:
2023-03-25
出版日期:
2023-05-05
发布日期:
2023-05-29
通讯作者:
李琪,麦立强
E-mail:swcshawn@163.com;liqi1@xhlab.cn;mlq518@whut.edu.cn
作者简介:
时文超(1996—),男,博士研究生,主要研究方向为水系锌离子电池体系的界面工程,E-mail:swcshawn@163.com;
基金资助:
Wenchao SHI1(), Yu LIU1, Bomian ZHANG1, Qi LI2(), Chunhua HAN1, Liqiang MAI1()
Received:
2023-02-22
Revised:
2023-03-25
Online:
2023-05-05
Published:
2023-05-29
Contact:
Qi LI, Liqiang MAI
E-mail:swcshawn@163.com;liqi1@xhlab.cn;mlq518@whut.edu.cn
摘要:
水系锌金属电池(AZMBs)由于价格低廉、安全性高,在大规模储能领域极具潜力。然而,锌金属在常规水系电解液中并不稳定,界面处容易产生锌枝晶、析氢和腐蚀等副反应,导致AZMBs循环寿命较短。其中,电解液添加剂可以有效调控锌负极界面的化学特性和反应过程,显著提升其界面稳定性,大幅延长AZMBs的循环寿命。因此,对电解液添加剂稳定锌负极的相关研究进行总结,并对目前存在的关键问题提出新的解决思路非常必要。本文通过对近期相关文献进行探讨,简要介绍了锌负极目前面临的主要挑战及其相关机理,重点阐述了电解液添加剂对锌负极界面的主要调控机制,包括设计静电屏蔽层、贫水双电层(EDL)、原位固体电解质界面(SEI)层以及调控锌离子溶剂化鞘层。此外,还对不同添加剂类型进行了分类讨论,包括阳离子型、阴离子型、有机小分子型、有机聚合物型和其他类型,并分析了其各自的调控机理和对电化学性能的影响。最后,本文还对电解液添加剂策略稳定锌负极的未来发展方向提出了展望。
中图分类号:
时文超, 刘宇, 张博冕, 李琪, 韩春华, 麦立强. 电解液添加剂稳定水系电池锌负极界面的研究进展[J]. 储能科学与技术, 2023, 12(5): 1589-1603.
Wenchao SHI, Yu LIU, Bomian ZHANG, Qi LI, Chunhua HAN, Liqiang MAI. Research progress and prospect on electrolyte additives for stabilizing the zinc anode interface in aqueous batteries[J]. Energy Storage Science and Technology, 2023, 12(5): 1589-1603.
图6
(a) 加入和不加入聚合物添加剂的不同水电解质中的键合网络示意图[87];(b) 在不同聚合物添加剂的1 mol/L ZnSO4 水溶液中,在1 mA/cm2 、1 mAh/cm2 的测试条件下,Zn-Cu电池的库仑效率和循环性能[87];(c) 丝胶蛋白、丝素蛋白和具有不同构象和极性基团的肽分子之间的关系示意图,以及它们在AZMBs中作为电解液添加剂的应用[89];(d) 在电流密度为10 mA/cm2 时,含/不含丝肽的ZnSO4 电解质中Zn沉积形貌的原位光学观察[89];(e) 在含不同浓度的丝肽添加剂的ZnSO4 电解液中Zn-Cu电池的库仑效率[89];(f) 在含/不含丝肽的ZnSO4 电解液中Zn-Zn对称电池的循环性能[89]"
图7
(a) 添加和不添加GO添加剂时锌负极表面电场分布,矢量场描述了电场的方向[91];(b)~(c) 制备的石墨烯量子点TEM图和HRTEM(c中的插图)[92];(d) 云母衬底上GQDs的AFM图和初始线A-B对应的高度剖面[92];(e) 在2 mA/cm2 下,添加和不添加GQDs的Zn||Zn对称电池的长循环曲线和相应的电压曲线[92];(f) 在云母上的纯C3N4QDs(左)和在高定向热解石墨上ZnSO4 水系电解液中的C3N4QDs(右),插图为对应线条的高度轮廓[93];(g)~(o) 在100 μA/cm2 的电流密度下,含C3N4QDs (g)~(j) 和不含C3N4QDs(k)~(o) 的HOPG上Zn沉积的原位AFM图[93];(p) 使用[BMIM]OTF添加剂稳定锌沉积过程的原理图[95];(q) 在5 mA/cm2 和25 mAh/cm2 下的循环性能[95]"
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