锂电池百篇论文点评（2024.12.1—2025.1.31）

doi:10.19799/j.cnki.2095-4239.2025.0155

摘要/Abstract

摘要：

该文是一篇近两个月的锂电池文献评述，以“lithium”和“batter*”为关键词检索了 Web of Science 从 2024年12月 1日至 2025年1月 31日上线的锂电池研究论文，共有 5413 篇。首选采用BERTopic主题模型对其摘要文本进行分析，构建锂电池论文的研究主题图，再选择其中100 篇加以评论。正极材料的研究集中于高镍层状材料和尖晶石结构LiNi_0.5Mn_1.5O₄材料的掺杂改性、表面包覆、结构设计等。负极材料的研究重点包括硅基负极的结构设计和性能提升、金属锂负极的界面和体相结构设计。固态电解质的研究包括对聚合物、硫化物和卤化物及其复合固态电解质的结构设计以及相关性能研究。其他电解液和添加剂的研究则主要包括不同电解质和溶剂对各类电池材料体系适配的研究，以及对新的功能性添加剂的探索。对固态电池，正极材料的体相改性、表面包覆和合成方法、锂金属负极的界面构筑和三维结构设计、无负极集流体的界面修饰有多篇文献报道。此外，锂硫电池和锂空电池也备受关注。电极中的锂离子输运和失效机制、锂沉积形貌和SEI结构演变、全电池热失控分析，电解质对CEI组分影响的理论模拟以及优化制造工艺的论文也有多篇。

关键词: 锂电池, 正极材料, 负极材料, 电解质, 电池技术

Abstract:

This bimonthly review paper highlights a comprehensive overview of the latest research on lithium batteries. A total of 5413 online papers from December 1, 2024, to January 31, 2025, were examined through the Web of Science database. Firstly, the BERTopic topic model is used to analyze the abstract text and the research topic map of lithium battery papers was drawn. 100 papers were selected for highlighting in this review. The selected studies cover various aspects of lithium batteries. Cathode materials including Ni-rich layered oxides and LiNi_0.5Mn_1.5O₄ are improved by doping, surface coating, and micro structural modifications. The cycling performances of Si-based anode are enhanced by structural design. Great efforts have been devoted to interfacial and bulk structure design of lithium metal anode. Studies on solid-state electrolytes focus on the structure design and performances in polymer, sulfide, and halide electrolytes, as well as their composite forms. In contrast, liquid electrolytes are improved through optimal solvent and lithium salt design for different battery applications and incorporating novel functional additives. For solid-state batteries, the modification, surface coating and synthesis methods of cathode, interface construction and three-dimensional structural design of lithium metal anode, as well as the interface modification of current collectors for anode-free batteries are widely investigated. The structural design of cathode and liquid electrolyte for lithium-sulfur battery are helpful to extend its cycling life. In addition, lithium-sulfur and lithium-oxygen batteries have also garnered significant attention. There are also a few papers on the ion transport and degradation mechanisms in electrodes, lithium deposition morphology and SEI structural evolution in electrolytes, the analysis of thermal runaway of full batteries, the theoretical simulation of the impact of solvents on the components of the CEI, as well as optimizing the manufacturing processes.

Key words: lithium batteries, cathode material, anode material, electrolyte, battery technology

中图分类号:

TM 911

张新新, 岑官骏, 乔荣涵, 朱璟, 郝峻丰, 孙蔷馥, 田孟羽, 金周, 詹元杰, 闫勇, 贲留斌, 俞海龙, 刘燕燕, 周洪, 黄学杰. 锂电池百篇论文点评（2024.12.1—2025.1.31）[J]. 储能科学与技术, doi: 10.19799/j.cnki.2095-4239.2025.0155.

Xinxin ZHANG, Guanjun CEN, Ronghan QIAO, Jing ZHU, Junfeng HAO, Qiangfu SUN, Mengyu TIAN, Zhou JIN, Yuanjie ZHAN, Yong YAN, Liubin BEN, Hailong YU, Yanyan LIU, Hong ZHOU, Xuejie HUANG. Reviews of selected 100 recent papers for lithium batteries （Dec. 1, 2024 to Jan. 31, 2025）[J]. Energy Storage Science and Technology, doi: 10.19799/j.cnki.2095-4239.2025.0155.

图/表 1

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