储能科学与技术 ›› 2024, Vol. 13 ›› Issue (7): 2192-2205.doi: 10.19799/j.cnki.2095-4239.2024.0559
李泽珩1,2(), 徐磊3, 姚雨星1, 闫崇3, 翟喜民4, 郝雪纯4, 陈爱兵5, 黄佳琦3, 别晓非4, 孙焕丽4, 范丽珍6, 张强1,7,8()
收稿日期:
2024-06-21
修回日期:
2024-07-01
出版日期:
2024-07-28
发布日期:
2024-07-23
通讯作者:
张强
E-mail:zehengli@zju.edu.cn;zhang-qiang@mails.tsinghua.edu.cn
作者简介:
李泽珩(1992—),男,博士,研究员,研究方向为锂电池,E-mail:zehengli@zju.edu.cn;
基金资助:
Zeheng LI1,2(), Lei XU3, Yuxing YAO1, Chong YAN3, Ximin ZHAI4, Xuechun HAO4, Aibing CHEN5, Jiaqi HUANG3, Xiaofei BIE4, Huanli SUN4, Lizhen FAN6, Qiang ZHANG1,7,8()
Received:
2024-06-21
Revised:
2024-07-01
Online:
2024-07-28
Published:
2024-07-23
Contact:
Qiang ZHANG
E-mail:zehengli@zju.edu.cn;zhang-qiang@mails.tsinghua.edu.cn
摘要:
锂离子电池作为便携式电子产品和电动汽车的“心脏”,在推动人类社会的无化石燃料化中发挥着至关重要的作用。然而,在低温条件下(0 ℃及以下)充电时,锂离子电池电极极化急剧增大,导致了严重的析锂问题。通过合理设计低温电解液,降低低温充电时电极极化,并构建稳定的电解液-电极界面,可以有效遏制析锂及其对锂离子电池带来的不利影响。本文首先阐释了低温下锂离子电池析锂的形成机制,并指出低温电解液的设计是改善锂离子电池低温析锂行为的有效途径。接着,本文进一步介绍了缓解低温析锂问题的几种电解液设计策略,包括降低去溶剂化能垒的弱溶剂化电解液和共嵌入电解液、衍生低阻抗固态电解质界面膜(SEI)的局部高盐电解液以及钝化析锂的羧酸酯基高盐电解液,同时比较了这些策略的优劣势。最后,结合现有研究成果,展望了电解液调控低温析锂行为的未来研究方向,提出了发展实时析锂预警方法、采用实用化条件评估电解液抑制低温析锂能力以及设计兼顾电化学动力学和界面稳定性的高比能硅碳负极用低温电解液,以望实现低温锂离子电池的高容量发挥和长循环寿命。
中图分类号:
李泽珩, 徐磊, 姚雨星, 闫崇, 翟喜民, 郝雪纯, 陈爱兵, 黄佳琦, 别晓非, 孙焕丽, 范丽珍, 张强. 电解液改善锂离子电池低温析锂研究进展[J]. 储能科学与技术, 2024, 13(7): 2192-2205.
Zeheng LI, Lei XU, Yuxing YAO, Chong YAN, Ximin ZHAI, Xuechun HAO, Aibing CHEN, Jiaqi HUANG, Xiaofei BIE, Huanli SUN, Lizhen FAN, Qiang ZHANG. A review of electrolyte reducing lithium plating in low-temperature lithium-ion batteries[J]. Energy Storage Science and Technology, 2024, 13(7): 2192-2205.
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