Recent advances in preparation of MOF-derived porous carbon-based materials and their applications in anodes of lithium-ion capacitors

doi:10.19799/j.cnki.2095-4239.2024.0050

Abstract

Abstract:

Lithium-ion capacitors represent novel power storage devices amalgamating the features of both lithium-ion batteries and supercapacitors. However, the sluggish dynamics of the lithium-ion capacitor's battery-type negative electrode, compared to the capacitor-type positive electrode, lead to a diminished power density and compromised cycle stability. Notably, porous carbon-based materials derived from metal-organic frameworks (MOFs) have emerged as a focal point in electrochemical energy storage research owing to their expansive specific surface area, porous structure, and exceptional chemical stability. This study analyzes the challenges associated with electrode materials of lithium-ion capacitors and elucidates the energy storage mechanism of lithium-ion capacitors. Subsequently, the influence of carbonization temperature and heat treatment time on the physicochemical properties of MOF-derived porous carbon-based materials is examined. Moreover, diverse products generated through the carbonization process are discussed. Furthermore, the advancements in utilizing MOF-derived porous carbon-based materials in lithium-ion capacitors are reviewed. Finally, the crucial role of composite or doping modifications with other carbon materials in improving the power and energy densities for anode materials of lithium-ion capacitors is emphasized.

Key words: lithium-ion capacitors, anode materials, metal-organic framework, porous carbon materials

CLC Number:

TM 911

Yanyan KONG, Xiong ZHANG, Yabin AN, Chen LI, Xianzhong SUN, Kai WANG, Yanwei MA. Recent advances in preparation of MOF-derived porous carbon-based materials and their applications in anodes of lithium-ion capacitors[J]. Energy Storage Science and Technology, 2024, 13(8): 2665-2678.

Figures/Tables 7

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Table 1

References 61

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类型	MOF 前驱体	衍生负极材料	正极材料	电压窗口/V	最高能量密度/(Wh/kg) @对应功率密度/(kW/kg)	最高功率密度/(kW/kg) @对应能量密度/Wh/kg	电流密度/(A/g) @循环次数	循环容量保持率	参考文献
类型一	Fe-BTC	OLC	AC	2.2～3.8	195@0.138	17.717@92	1@4000	61.5%	[49]
	Zn-MOF	Z-T-PC	PC	1.5～4	95.8@0.2644	46@54.6	2@5000	83.67%	[51]
	ZIF-8	HCF-2	a-HCF-2	1～4.5	162@0.48	15.8@114.5	5@15000	76%	[52]

类型二	ZIF-67	Co@N-C	HPC	0～4	125.28@0.2	10@38.33	1@1000	91.74%	[60]
	Mn-MOF	MnO₂ @C-NS	NPCs	0.01～4	166@0.55	3.9@49.3	1@5000	91%	[53]
	CoZn-MOF	Co₃ZnC@NC	MPC	1.0～4.5	141.4@0.275	10.3@15.2	1@1000	80%	[14]
	CoZn-MOF	Co₃ZnC@NC	预锂化石墨	1～3	67.1@0.12	4.1@1.48	0.1@1000	—	[61]

类型三	Mn-MOF	Mn₂SnO₄@C	CSBC	1.5～4.5	217.9@0.21	21@25	2@5000	79%	[58]
	ZIF-67	CoTe₂@N-C	HPC	0～4	144.5@0.2	10@38.89	1@1000	90.95%	[59]
	ZIF-67	CoSn _x @CPAN	PDPC	1.5～4.2	143@0.285	22.8@41	2@5000	82.9%	[57]
	钼基MOF	MoO₂@rGO	PANI@rGO	1.25～4.5	241.7@0.2875	28.75@117.8	5@10000	96%	[56]

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