Effect of carbon sequestration on the performance of waste concrete shape-stable phase change composites

doi:10.19799/j.cnki.2095-4239.2023.0685

Abstract

Abstract:

In order to fully resource the use of waste concrete to capture and store CO₂, this paper utilizes waste concrete for carbon capture, and seven composite phase change heat storage materials with different mass ratios were prepared by using carbon consolidated and unconsolidated waste. Results indicate that the carbon sequestration efficiency of the waste concrete was as high as 24.7% under the specific experimental conditions. The latent heat of melting of the shape-stable phase change composites prepared by carbon sequestration was higher than that before carbon sequestration after adding the same mass fraction of phase change material. The compressive strength of SS2 was as high as 121.54 MPa, and the compressive strengths of both the carbon sequestered waste concrete and shape-stable phase change composites were significantly increased, with the highest thermal conductivity [0.648 W/(m·K)] being lower than that of the un-sequestered sample [0.884 W/(m·K)]. The shape-stable phase change composites before and after carbon sequestration had good chemical compatibility among the components, and the phase change materials were densely bonded with the skeleton materials.

Key words: waste concrete, carbon sequestration, skeleton material, shape-stable phase change composites, energy storage

CLC Number:

TB 332

Xi TIAN, Yaxuan XIONG, Jing REN, Yanqi ZHAO, Shihao JIN, Shuo LI, Yang YANG, Yulong DING. Effect of carbon sequestration on the performance of waste concrete shape-stable phase change composites[J]. Energy Storage Science and Technology, 2023, 12(12): 3709-3719.

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样品	废弃混凝土/%	NaNO₃/%	烧结后形貌	样品	固碳后废弃混凝土/%	NaNO₃/%	烧结后形貌
SS1	70	30	成型良好	C-SS1	70	30	成型良好
SS2	60	40	成型良好	C-SS2	60	40	成型良好
SS3	55	45	成型较好	C-SS3	55	45	成型良好
SS4	50	50	成型较好，轻微熔盐泄漏	C-SS4	50	50	有开裂趋势
SS5	45	55	样品表面鼓包	C-SS5	45	55	样品开裂
SS6	40	60	样品胀大	C-SS6	40	60	样品开裂
SS7	30	70	样品严重损坏	C-SS7	30	70	样品变形

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