Review on solid state lithium-sulfur batteries with sulfide solid electrolytes

doi:10.12028/j.issn.2095-4239.2017.0033

Energy Storage Science and Technology ›› 2017, Vol. 6 ›› Issue (3): 464-478.doi: 10.12028/j.issn.2095-4239.2017.0033

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Review on solid state lithium-sulfur batteries with sulfide solid electrolytes

SUN Yingzhi ^{1, 2,} HUANG Jiaqi ^{1, 3}, ZHANG Xueqiang¹, ZHANG Qiang¹

¹Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China; ²School of Materials Science and Engineering, Tsinghua University, Beijing 100084, China; ³Advanced Research Institute for Multidisciplinary Science, School of Materials Science & Engineering, Beijing Institute of Technology, Beijing 100081, China

Received:2017-03-29 Revised:2017-04-01 Online:2017-05-01 Published:2017-05-01

Abstract

Abstract:

The development of electronic devices, such as portable electronics, electric vehicles and smart grids, brings new requirements and challenges to electrochemical energy storage system. Solid state lithium-sulfur batteries have attracted much attention for their high theoretical energy density and safety properties. Owning to high ionic conductivity and excellent interface contact, sulfide solid electrolytes are suitable for solid state lithium-sulfur batteries. This review summarizes the recent progress of solid state lithium-sulfur batteries with sulfide solid electrolytes. It focuses on the properties of sulfide solid electrolytes, the formation of efficient carrier pathways on the cathode side, and the stable lithium/electrolyte interfaces on the anode side. The future development directions of solid state lithium-sulfur batteries with sulfide solid electrolytes are also prospected.

Key words: lithium sulfur battery, solid electrolyte, ionic conductivity, sulfide, lithium metal anode

SUN Yingzhi, HUANG Jiaqi, ZHANG Xueqiang, ZHANG Qiang. Review on solid state lithium-sulfur batteries with sulfide solid electrolytes[J]. Energy Storage Science and Technology, 2017, 6(3): 464-478.

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Review on solid state lithium-sulfur batteries with sulfide solid electrolytes

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