锂电池百篇论文点评（2024-12-01—2025-01-31）

doi:10.19799/j.cnki.2095-4239.2025.0155

储能科学与技术 ›› 2025, Vol. 14 ›› Issue (3): 1310-1330.doi: 10.19799/j.cnki.2095-4239.2025.0155

• 热点点评 • 上一篇

锂电池百篇论文点评（2024-12-01—2025-01-31）

张新新¹(), 岑官骏¹, 乔荣涵¹, 朱璟¹, 郝峻丰¹, 孙蔷馥¹, 田孟羽², 金周², 詹元杰², 闫勇², 贲留斌², 俞海龙¹, 刘燕燕¹, 周洪³, 黄学杰¹^,²()

^1.中国科学院物理研究所，北京 100190
^2.松山湖材料实验室，广东东莞 523890
^3.中国科学院武汉文献情报中心，湖北武汉 430071

收稿日期:2025-02-22 出版日期:2025-03-28 发布日期:2025-04-28
通讯作者: 黄学杰 E-mail:zhangxinxin223@mails.ucas.ac.cn;xjhuang@iphy.ac.cn
作者简介:张新新（1999—），女，博士研究生，研究方向为锂离子电池，E-mail：zhangxinxin223@mails.ucas.ac.cn；
基金资助:
支持单位：中国科学院物理研究所、过程工程研究所、大连化学物理研究所储能技术部、工程热物理研究所、上海硅酸盐研究所，中国电力科学院，清华大学化学工程系、工程物理系，比亚迪汽车工业有限公司、东洋纺、泰思泰克、宇电科技、昊诚锂电、科华数能、领声科技、中储国能、中科海钠、新威尔、卫蓝新能源、亿纬锂能、宁德时代新能源、新宙邦、赣锋锂业、天齐锂业、湖南立方新能源等

Reviews of 100 selected recent papers on lithium batteries (December 1, 2024 to January 31, 2025)

Xinxin ZHANG¹(), Guanjun CEN¹, Ronghan QIAO¹, Jing ZHU¹, Junfeng HAO¹, Qiangfu SUN¹, Mengyu TIAN², Zhou JIN², Yuanjie ZHAN², Yong YAN², Liubin BEN², Hailong YU¹, Yanyan LIU¹, Hong ZHOU³, Xuejie HUANG¹^,²()

^1.Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China
^2.Songshan Lake Materials Laboratory, Dongguan 523890, Guangdong, China
^3.National Science Library (Wuhan), Chinese Academy of Sciences, Wuhan 430071, Hubei, China

Received:2025-02-22 Online:2025-03-28 Published:2025-04-28
Contact: Xuejie HUANG E-mail:zhangxinxin223@mails.ucas.ac.cn;xjhuang@iphy.ac.cn

摘要/Abstract

摘要：

该文是一篇近两个月的锂电池文献评述，以“lithium”和“batter*”为关键词检索了Web of Science从2024年12月1日至2025年1月31日上线的锂电池研究论文，共有5413篇。首选采用BERTopic主题模型分析其摘要文本，构建锂电池论文的研究主题图，再选择其中100篇加以评论。正极材料的研究集中于高镍层状材料和尖晶石结构LiNi_0.5Mn_1.5O₄材料的掺杂改性、表面包覆、结构设计等。负极材料的研究重点包括硅基负极的结构设计和性能提升、金属锂负极的界面和体相结构设计。固态电解质的研究包括对聚合物、硫化物和卤化物及其复合固态电解质的结构设计以及相关性能研究。其他电解液和添加剂的研究则主要包括不同电解质和溶剂对各类电池材料体系适配的研究，以及对新的功能性添加剂的探索。对固态电池，正极材料的体相改性、表面包覆和合成方法、锂金属负极的界面构筑和三维结构设计、无负极集流体的界面修饰有多篇文献报道。此外，锂硫电池和锂空电池也备受关注。电极中的锂离子输运和失效机制、锂沉积形貌和SEI结构演变、全电池热失控分析，电解质对CEI组分影响的理论模拟以及优化制造工艺的论文也有多篇。

关键词: 锂电池, 正极材料, 负极材料, 电解质, 电池技术

Abstract:

This bimonthly review provides a comprehensive overview of recent research on lithium batteries. A total of 5413 online papers published between December 1, 2024 and January 31, 2025 were examined using the Web of Science database. Using the BERTopic model, the abstract texts were analyzed, and a research topic map for lithium battery studies was generated. From these, 100 papers were selected for in-depth discussion. The selected studies covered various aspects of lithium batteries. Research on cathode materials, including Ni-rich layered oxides and LiNi_0.5Mn_1.5O₄, focuses on improvements through doping, surface coating, and microstructural modifications. The cycling performances of Si-based anodes were enhanced through structural design. Considerable efforts have been devoted to interfacial and bulk structure design for lithium metal anodes. Studies on solid-state electrolytes examined structural design and performance in polymer, sulfide, and halide electrolytes as well as their composite forms. In contrast, liquid electrolytes were improved through optimized solvent and lithium salt designs for different battery applications and the incorporation of novel functional additives. For solid-state batteries, studies have explored cathode modification, surface coating, and synthesis methods as well as interface construction and three-dimensional structural design for lithium metal anodes. Interface modifications of current collectors for anode-free batteries have also been widely investigated. In lithium-sulfur batteries, the structural design of the cathode and liquid electrolyte contributes to extended cycle life. In addition, lithium-sulfur and lithium-oxygen batteries have garnered considerable attention. Other studies have investigated ion transport and degradation mechanisms in electrodes, lithium deposition morphology, and solid electrolyte interphase evolution. Research has also addressed thermal runaway analysis in full batteries, theoretical simulations of solvent effects on the cathode electrolyte interphase, and optimization of manufacturing processes.

Key words: lithium batteries, cathode material, anode material, electrolyte, battery technology

中图分类号:

TM 911

张新新, 岑官骏, 乔荣涵, 朱璟, 郝峻丰, 孙蔷馥, 田孟羽, 金周, 詹元杰, 闫勇, 贲留斌, 俞海龙, 刘燕燕, 周洪, 黄学杰. 锂电池百篇论文点评（2024-12-01—2025-01-31）[J]. 储能科学与技术, 2025, 14(3): 1310-1330.

Xinxin ZHANG, Guanjun CEN, Ronghan QIAO, Jing ZHU, Junfeng HAO, Qiangfu SUN, Mengyu TIAN, Zhou JIN, Yuanjie ZHAN, Yong YAN, Liubin BEN, Hailong YU, Yanyan LIU, Hong ZHOU, Xuejie HUANG. Reviews of 100 selected recent papers on lithium batteries (December 1, 2024 to January 31, 2025)[J]. Energy Storage Science and Technology, 2025, 14(3): 1310-1330.

图/表 2

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82	YUN H, LEE E, HAN J, et al. Voltage noise failure induced by Li dendritic micro-penetration in all-solid-state Li-metal battery with composite solid electrolyte[J]. Advanced Energy Materials, 2024: 2404044. DOI: 10.1002/aenm.202404044.
83	CHEN B W, XU K, TANG L F, et al. In operando visualization of polymerized ionic liquid electrolyte migration in solid-state lithium batteries[J]. ACS Energy Letters, 2025, 10(1): 305-312. DOI: 10.1021/acsenergylett.4c02430.
84	MAITY A, SVIRINOVSKY-ARBELI A, BUGANIM Y, et al. Tracking dendrites and solid electrolyte interphase formation with dynamic nuclear polarization-NMR spectroscopy[J]. Nature Communications, 2024, 15(1): 9956. DOI: 10.1038/s41467-024-54315-w.
85	YU Z K, GAN C J, MIJAILOVIC A S, et al. Lithium dendrite deflection at mixed ionic-electronic conducting interlayers in solid electrolytes[J]. Advanced Energy Materials, 2024: 2403179. DOI: 10.1002/aenm.202403179.
86	ZHANG X, MAO S Y, HAN X B, et al. Online lithium plating detection based on charging internal resistance for lithium-ion batteries[J]. Journal of Energy Storage, 2025, 108: 115140. DOI: 10.1016/j.est.2024.115140.
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93	HUO H Y, BAI Y, BENZ S L, et al. Decoupling the effects of interface chemical degradation and mechanical cracking in solid-state batteries with silicon electrode[J]. Advanced Materials, 2025, 37(7): 2415006. DOI: 10.1002/adma.202415006.
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95	LEAU C, WANG Y, GERVILLIÉ-MOURAVIEFF C, et al. Tracking solid electrolyte interphase dynamics using operando fibre-optic infra-red spectroscopy and multivariate curve regression[J]. Nature Communications, 2025, 16(1): 757. DOI: 10.1038/s41467-024-55339-y.
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100	CHEN J F, FANG M D, WU Q, et al. Insights into the atomic mechanism of lithium-ion diffusion in Li₆PS₅Cl via a machine learning potential[J]. Chemistry of Materials, 2025, 37(2): 591-599. DOI: 10.1021/acs.chemmater.4c01152.

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锂电池百篇论文点评（2024-12-01—2025-01-31）

Reviews of 100 selected recent papers on lithium batteries (December 1, 2024 to January 31, 2025)

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